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  • Sulfadiazine/hydroxypropyl-beta-cyclodextrin host-guest system: Characterization, phase-solubility and molecular modeling.

Sulfadiazine/hydroxypropyl-beta-cyclodextrin host-guest system: Characterization, phase-solubility and molecular modeling.

Bioorganic & medicinal chemistry (2008-04-25)
Márcia Valéria Gaspar de Araújo, Elze Kelly Barbosa Vieira, Gilderman Silva Lázaro, Leila Souza Conegero, Luís Eduardo Almeida, Ledjane Silva Barreto, Nivan Bezerra da Costa, Iara F Gimenez
ABSTRACT

In this work we prepared and characterized an inclusion complex of the dihydropteroate synthase inhibitor sulfadiazine (SDZ) in 2-hydroxypropyl-beta-cyclodextrin (HPBCD). From the phase-solubility diagram we observed an increase in the water solubility of the drug, calculating a binding constant of 1879M(-1). The inclusion mode involves a NH(2)-in orientation of the drug in the HPBCD cavity, according to the 2D NMR (ROESY) data and confirmed by molecular modeling using the semiempirical PM6 and RM1 methods.

MATERIALS
Product Number
Brand
Product Description

Supelco
Sulfadiazine, VETRANAL®, analytical standard
Sigma-Aldrich
Sulfadiazine, 99.0-101.0%