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Polyimide (PI) is a novel organic material for new generation energy storage devices. PI can be a potential high-power electrode material for rechargeable battery and super-capacitor applications because its faster redox kinetics than inorganic materials. PI-graphene nanocomposite takes advantages of graphene′s excellent electronic conductivity and high surface area, which addresses the issues of PI′s electronic insulation and further improve its utilization. With the added benefit of high safety, flexibility and easy processability, PI composited graphene nanocomposites would penetrate the field of energy storage in the near future.